Opening ZIF-8: A Catalytically Active Zeolitic Imidazolate Framework of Sodalite Topology with Unsubstituted Linkers

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Opening ZIF-8: a catalytically active zeolitic imidazolate framework of sodalite topology with unsubstituted linkers.

A zeolitic imidazolate framework material of SOD topology possessing primarily unsubstituted imidazolate (im) linkers has been synthesized via solvent-assisted linker exchange (SALE) of ZIF-8. The structure of the new material, SALEM-2, has been confirmed through (1)H NMR and powder and single-crystal X-ray diffraction. SALEM-2 is the first example of a porous Zn(im)(2) ZIF possessing a truly z...

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ژورنال

عنوان ژورنال: Journal of the American Chemical Society

سال: 2012

ISSN: 0002-7863,1520-5126

DOI: 10.1021/ja308786r